Granular materials

Tilo Finger, David Fischer, Frank Rietz, Sandra Wegner, Kirsten Harth, Ralf Stannarius

nematic_EHC

Axial segregation of granular material in a long horizontal rotating drum

  • Granular mixtures of particles which differ in size, density or surface roughness show the tendency to segregate under a wide variety of flow conditions
  • A typical example is the segregation along the axis of a partially filled horizontally rotating drum
  • The system shows a very interesting dynamics:
    • After a few rotations the small grains forms a core along the axis of the drum (radial segregation).
    • A few rotations later, this core becomes unstable and a stripe pattern appears (axial segregation).
    • After the formation of the stripe pattern a so-called coarsening sets in. This means that individual stripes shrink until they vanish, while other stripes grow in size.
  • Until now, the coarsening dynamic is only poorly understood .
Bilda0001.jpg initial mixed state
Bilda0050.jpg after 500 rotations
Bildb0400.jpg after 23000 rotations
  • Advantages of the system compared to other segregation experiments:
    • The energy can be supplied continuously and uniformly over arbitrarily long time periods.
    • The stripe pattern can be observed straightforwardly.
    • The time evolution of the visible stripe pattern can be mapped in space-time plots.
  • Elucidation of the 3-dimensional particle distribution is one important prerequisite to understand the mechanism of coarsening.
  • The 3D particle distribution is investigated non-invasively by Magnetic Resonance Imaging (MRI). Experiments were performed in collaboration with the LIN Magdeburg [Finger2006,Finger2007,Fischer2009,Naji2009].

Our particular topic of interest is the coarsening of the stripe patterns, the distribution and the axial transport of grains:
  • What are the scaling laws of the coarsening process?
  • What is the drivingl mechanism of coarsening?
  • How can the axial grain transport be described?
  • What is the internal structure of the segregation pattern?
spacetime.jpg
Space time plot of a striped segregation pattern (left), the cylindrical drum of 38 mm diameter and 1m length is half filled with a 50:50 mixture of 1.5 and 0.55 mm diameter glass beads. The characteristic feature is the logarithmic decay of the number of segregation stripes. In the investigated mixtures, stripes of small beads lose material to neighboring stripes or gain material from there.
37_8.jpg



Example: experimental cross section (sagittal section, along the vertical midplane of the tube). The tube is filled with glass beads in water. Bright areas reflect the proton signal from the surrounding water. One acknowledges two stripes of the small bead species separated by a band of large beads. In the core, one observes a channel of small beads connecting the two outer stripes. This channel is essential for the stripe dynamics.
glycerol
Influence of the interstitial fluid:  Space-time plots of the coarsening of segregation patterns, mixture of glass beads with 1.5 mm and 0.55 mm diameter. The granulate is embedded in a 80% glycerol in water mixture (left) and a 40% glycerol in water mixture (right). The viscosity of the embedding fluid has little influence on the dynamics of the stripe pattern [Finger2007] 

Segregation in rotating spherical mixers

A spherical container (37 mm diameter) filled with a bidisperse mixture of spherical beads (0.5 mm and 1.5 mm diameter) is rotated about a horizontal axis at rotation rates of several rpm. The initial fill level determines the type of segregation pattern that is formed. At low fill levels, small beads occupy the poles while large beads occupy the equatorial zone. At high fill levels, the positions of stripes of small and large beads appear interchanged, small beads occupy the equatorial zone, large beads the polar zones. The mechanism is not fully understood yet [Naji2009].
two regimes
Two regimes are observed in a spherical mixer that rotates about a horizontal axis:
  • when the fill level is below 30%, the small beads occupy the lateral zones and large beads are located in the central zone
  • when the fill level is above 50%, the large beads accumulate in the lateral zones and small beads form the central zone
  • at fill levels around 40%, a transition region is found. Often, only two zones are formed there
low fill level
Vertical MRI slices of the SLS (small-large-small) segregation pattern at low fill levels. Slice a contains the rotation axis, slices b-e are normal to the rotation axis. Water appears bright in the images, the beads black. At the top, an entrapped air bubble is seen. A core of small beads links the two polar segregation bands.
high fill level
Vertical MRI slices of the LSL (large-small-large) segregation pattern at high fill levels. Slice a contains the rotation axis, slices b-e are normal to the rotation axis. Conical tongues of small beads extend into the polar bands of large beads.

Diffusion of granular material in a long horizontal rotating drum

Measurement of the particle dynamics in a rotating mixer [Fischer2009]
  • preparation of a 'pulse' of grains in a rotating mixer with 50% fill height (right), a slice of large/small glass beads is prepared initially in a bed of small/large beads
  • Diffusion of glass beads observed optically, view onto the flowing layer of the rotating cylindrical tube (bottom left). Small beads (black) diffuse axially into regions of large beads (light green), images were taken after a) 0 rotations, b) 30 rotations and c) 300 rotations.
  • MRI slices of the cylinder (bottom right), the bright regions contain water, the glass beads appear as black shadows. From the particle positions, the time dependent axial distribution and the character of the diffusion are obtained. 
pulse
optics MRI

Convection and segregation in rotating flat containers

A flat container (approximately 5 - 10 particle diameters thick, see image) is filled with a bidisperse mixture of grains and rotated about a horizontal axis. We observe two different scenarios, depending upon the fill level. At low fill level, chute flow leads to a lateral segregation into stationary or traveling stripes, coarsening of the stripe pattern can occur. In cells with high fill level we observe convective patterns. setup
granular convection
Convection rolls in a cell with high fill level [Rietz2008,Rietz2012NJP]
single rolls
In containers with aspect ratio close to one, single rolls form. In contrast to multiple rolls in cells with larger aspect ratios, these single rolls exhibit fluctuations, cessations and spontaneous reversal of the convective flow [Rietz2012PRL].
traveling rolls
In cells with low fill ratio, the granulate segregates into lateral stripes. These stripes can spontaneously form or decay, merge, and move in axial direction. Traveling wave patterns have been observed [Rietz2012PRE]. These patterns can show quasi-periodicity over long periods. During long-term experiments in an individual cell, the spontaneous transition between different periodic traveling wave patterns can take place spontaneously.
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Shear zone refraction in layered granulate

in collaboration with T. Börzsönyi (Hungarian Academy of Sciences, Budapest)
gedankenexperiment
Gedankenexperiment [Börzsönyi2011], two layers of grains, the upper one with low friction, the lower one with high friction:
When the bottom (u-shaped) slider is moved respective to the upper counterpart, a shear zone separates material moving with the bottom slider from material remaining at rest with the top slider. This shear zone selects a shape where it minimizes friction,. Similar to Fermat's principle in optics. In first approximation, the integral of the friction coefficient along the shear zone is minimized. The result is a shear zone geometry analogous to Snellius's law of refraction and reflection in optics.
closed system
experimentally determined shear zone geometries in vertically stacked layers of korundum (high friction, bottom) and glass beads (low friction, top). The zone geometries were determined by excavation of color-labeled layers
open system
experimentally determined shear zone geometries in horizontally stacked layers of korundum (high friction, left) and glass beads (low friction, right). The zone geometries were determined by excavation of color-labeled layers (a-c) and MRI imaging of poppy seed tracers (d-f)

Orientational order and shear alignment of anisometric grains

Anisometric grains can be aligned by shear flow. We study the orientational order and shear alignment of anisometric grains by means of optical techniques and three-dimensional tomographic imaging (X-ray Computed Tomography and Magnetic Resonance Imaging)
split-bottom cell
Shear experiments in a container with split-bottom geometry: A disk on the container bottom with a smaller radius than that of the cylindrical container is rotated. The granulate in the container (rice in the picture above) is sheared and it forms a localized shear zone. Rodlike or elongated cylindrical grains align in a preferential orientation, a few degrees off the shear flow direction. [Börzsönyi2012PRL,Börzsönyi2012PRE]
X-ray CT
X-ray CT of an ensemble of sheared wooden cylinders (25 mm length, 5 mm diameter). Image a) shows the shear geometry of the cylindrical split-bottom cell, the shear zone (red) and the section of the CT image (dashed black box); images b) and c) show reconstructions of the particles from the CT data [Wegner2012].

Granular gases of anisometric grains

A granular gas of rodlike grains is studied under weak excitation, to identify its statistical properties. An interesting question in such an ensemble is the test of the equipartition of mechanical energy on the different translational and rotational degrees of freedom.
The rods of about 12 mm length and 1.3 mm diameter are contained in a cuboid box with dimensions of 8 x 10 x 6 cm. Three walls of the box vibrate with 30 Hz frequency and a vibration amplitude of the order of 2 mm (image).
The experiment was performed in a suborbital rocket that provided approximately 70 seconds of microgravity.

The first experiment was designed and performed within the REXUS-10 campaign of DLR, SNSB and ESA, project GAGa (Granular Anisotropic Gases). The team members GAGa were K. Harth, T. Trittel, U. Kornek, U. Strachauer, K. Will, and S. Höme. Data evaluation and modeling are in progress.
GAGa box


T. Finger, A. Voigt, J. Stadler, H.G. Niessen, L. Naji, and R. Stannarius. Coarsening of axial segregation patterns of slurries in a horizontally rotating drum. Phys. Rev. E, 74 031312, (2006).
T. Finger and R. Stannarius. Influence of the interstitial liquid on segregation patterns of granular slurries in a rotating drum. Phys. Rev. E, 75 031308, (2007).
D. Fischer, T. Finger, F. Angenstein, and R. Stannarius. Diffusive and subdiffusive axial transport of granular material in rotating mixers. Phys. Rev. E, 80 061302, (2009).
L. Naji and R. Stannarius. Axial and radial segregation of granular mixtures in a rotating spherical container. Phys. Rev. E, 79 031307, (2009).
T. Börzsönyi, T. Unger, B. Szabo, S. Wegner, F. Angenstein, and R. Stannarius. Reflection and exclusion of shear zones in inhomogeneous granular materials. Soft Matter, 7 8330, (2011).
T. Börzsönyi, B. Szabo, G. Törös, S. Wegner, J. Török, E. Somfai, T. Bien, and R. Stannarius. Orientational order and alignment of elongated particles induced by shear. Phys. Rev. Lett., 108 228302, (2012).
T. Börzsönyi, B. Szabo, S. Wegner, K. Harth, J. Török, E. Somfai, T. Bien, and R. Stannarius. Shear induced alignment and dynamics of elongated granular particles. Phys. Rev. E, 86 051304, (2012).
S.Wegner, T. Börzsöny, T. Bien, G. Rose, and R. Stannarius. Alignment and dynamics of elongated cylinders under shear. Soft Matter, 8 10950, (2012).
F. Rietz and R. Stannarius. On the brink of jamming: Granular convection in densely filled containers. Phys. Rev. Lett., 100 078002, (2008).
F. Rietz and R. Stannarius. Convection and segregation in a flat rotating sandbox. New J. Phys.,14 015001, (2012).
F. Rietz and R. Stannarius. Oscillations, cessations and circulation reversals of granular convection in a densely filled rotating container. Phys. Rev. Lett., 108 118001, (2012).
F. Rietz and R. Stannarius. Transitions between multiple attractors in a granular experiment. Phys. Rev. E., 85 040302(R), (2012).


last modified Feb. 21, 2013, R. Stannarius